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题名

Post-growth Fe deposition on the superconductivity of monolayer FeSe films on SrTi O3-δ

作者
通讯作者Pan,Minghu; Wang,Lili
发表日期
2022-06-01
DOI
发表期刊
EISSN
2475-9953
卷号6期号:6
摘要
The superconductivity in bulk FeSe depends sensitively on the stoichiometry, ditto for the monolayer FeSe films grown on SrTiO3-δ and other substrates. To tune the stoichiometry, we deposit Fe onto monolayer FeSe films after epitaxial growth. Using in situ low-temperature scanning tunneling microscopy/spectroscopy, we find that the postdeposited Fe atoms incorporate into monolayer films and combine with excess Se to form FeSe, with an upper coverage limit of ∼0.4 unit-cell. Consequently, the superconducting gap concentrates in 10 to 12 meV. The work demonstrates a simple method for stoichiometry tuning and improving the spatial uniformity of monolayer FeSe films. Compared with the gap of ∼15 to 20 meV for the annealed films, the smaller superconducting gap indicates weakened FeSe-TiO2 coupling due to interfacial Se atom substitution.
相关链接[Scopus记录]
收录类别
SCI ; EI
语种
英语
学校署名
其他
WOS记录号
WOS:000817850500001
EI入藏号
20222912368503
EI主题词
Binary alloys ; Iron ; Scanning tunneling microscopy ; Selenium ; Selenium compounds ; Stoichiometry ; Superconducting films ; Temperature ; Thin films ; Titanium dioxide
EI分类号
Iron:545.1 ; Nonferrous Metals and Alloys excluding Alkali and Alkaline Earth Metals:549.3 ; Thermodynamics:641.1 ; Superconducting Materials:708.3 ; Physical Chemistry:801.4 ; Inorganic Compounds:804.2
Scopus记录号
2-s2.0-85134081061
来源库
Scopus
引用统计
被引频次[WOS]:5
成果类型期刊论文
条目标识符//www.snoollab.com/handle/2SGJ60CL/401642
专题理学院_物理系
作者单位
1.State Key Laboratory of Low-Dimensional Quantum Physics,Department of Physics,Tsinghua University,Beijing,100084,China
2.School of Physics & Information Technology,Shaanxi Normal University,Xian,710119,China
3.Beijing Academy of Quantum Information Sciences,Beijing,100193,China
4.Department of Physics,Southern University of Science and Technology,Shenzhen,518055,China
推荐引用方式
GB/T 7714
Jiao,Xiaotong,Gong,Guanming,Zhang,Zhiyu,et al. Post-growth Fe deposition on the superconductivity of monolayer FeSe films on SrTi O3-δ[J]. Physical Review Materials,2022,6(6).
APA
Jiao,Xiaotong.,Gong,Guanming.,Zhang,Zhiyu.,Dong,Wenfeng.,Ding,Cui.,...&Xue,Qi Kun.(2022).Post-growth Fe deposition on the superconductivity of monolayer FeSe films on SrTi O3-δ.Physical Review Materials,6(6).
MLA
Jiao,Xiaotong,et al."Post-growth Fe deposition on the superconductivity of monolayer FeSe films on SrTi O3-δ".Physical Review Materials 6.6(2022).
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