中文版 | English
题名

Rate-dependent fracture of hydrogels due to water migration

作者
通讯作者Lu,Tongqing
发表日期
2022-10-01
DOI
发表期刊
ISSN
0022-5096
EISSN
1873-4782
卷号167
摘要
When a hydrogel deforms, the water molecules inside the hydrogel move together with the polymer network. At a particular time scale and length scale, the water migration within the hydrogel as well as the water exchange with the environment can greatly affect the deformation of the hydrogel. In this work, we study the rate-dependent fracture of hydrogels due to water migration both experimentally and theoretically. We build an experimental setup that can apply mechanical loads to hydrogel samples immersed in a liquid environment, water or oil. We apply monotonic load to hydrogel samples under different loading rates and find that the fracture stretch of hydrogel is highly dependent on the loading rate when the hydrogel is immersed in water, and is almost independent of the loading rate when the hydrogel is immersed in oil. We also apply step load to hydrogel samples and find that the hydrogel immersed in water is more susceptible to delayed fracture than that immersed in oil. We adopt the large deformation theory incorporating water migration developed by Hong et al. (2008) and use finite element software to calculate the deformation and fracture of hydrogels under the two types of environmental conditions. The numerical calculations show that at the time scale and length scale used in the experiment, the water migration satisfies the small-scale swelling condition of fracture. When the hydrogel is immersed in water, the water molecules can exchange with the environment under different loading rates. When the hydrogel is immersed in oil, the water molecules can hardly move in or out of the hydrogel. The theoretical predictions explain the experimental results.
关键词
相关链接[Scopus记录]
收录类别
SCI ; EI
语种
英语
学校署名
其他
资助项目
National Natural Science Foundation of China[11922210, 11732012];National Natural Science Foundation of China[11972015];
WOS研究方向
Materials Science ; Mechanics ; Physics
WOS类目
Materials Science, Multidisciplinary ; Mechanics ; Physics, Condensed Matter
WOS记录号
WOS:000853876300002
出版者
EI入藏号
20223012410826
EI主题词
Deformation ; Fracture ; Loading ; Molecules
EI分类号
Materials Handling Methods:691.2 ; Colloid Chemistry:801.3 ; Chemical Products Generally:804 ; Atomic and Molecular Physics:931.3 ; Materials Science:951
ESI学科分类
ENGINEERING
Scopus记录号
2-s2.0-85134640766
来源库
Scopus
引用统计
被引频次[WOS]:11
成果类型期刊论文
条目标识符//www.snoollab.com/handle/2SGJ60CL/359522
专题工学院_力学与航空航天工程系
作者单位
1.State Key Lab for Strength and Vibration of Mechanical Structures. Department of Engineering Mechanics,Xi'an Jiaotong University,Xi'an,710049,China
2.Department of Mechanics and Aerospace Engineering,Southern University of Science and Technology,Shenzhen,518055,China
推荐引用方式
GB/T 7714
Yang,Yan,Guo,Haoyu,Du,Zhenjiang,et al. Rate-dependent fracture of hydrogels due to water migration[J]. JOURNAL OF THE MECHANICS AND PHYSICS OF SOLIDS,2022,167.
APA
Yang,Yan,Guo,Haoyu,Du,Zhenjiang,Hong,Wei,Lu,Tongqing,&Wang,Tiejun.(2022).Rate-dependent fracture of hydrogels due to water migration.JOURNAL OF THE MECHANICS AND PHYSICS OF SOLIDS,167.
MLA
Yang,Yan,et al."Rate-dependent fracture of hydrogels due to water migration".JOURNAL OF THE MECHANICS AND PHYSICS OF SOLIDS 167(2022).
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