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题名	Molecular mechanism of abnormally large nonsoftening deformation in a tough hydrogel
作者	Ye，Ya Nan 1; Cui，Kunpeng 2; Hong，Wei1,3 ; Li，Xueyu 1; Yu，Chengtao 4; Hourdet，Dominique 1,5; Nakajima，Tasuku 1,6,7; Kurokawa，Takayuki 1,7; Gong，Jian Ping 6,7,8
发表日期	2021-04-06
DOI	10.1073/pnas.2014694118
发表期刊	Proceedings of the National Academy of Sciences of the United States of America 影响因子和分区
EISSN	1091-6490
卷号	118 期号:14
摘要	Tough soft materials usually show strain softening and inelastic deformation. Here, we study the molecular mechanism of abnormally large nonsoftening, quasi-linear but inelastic deformation in tough hydrogels made of hyperconnective physical network and linear polymers as molecular glues to the network. The interplay of hyperconnectivity of network and effective load transfer by molecular glues prevents stress concentration, which is revealed by an affine deformation of the network to the bulk deformation up to sample failure. The suppression of local stress concentration and strain amplification plays a key role in avoiding necking or strain softening and endows the gels with a unique large nonsoftening, quasi-linear but inelastic deformation.
关键词	hyperconnective network large quasi-linear deformation molecular glue nonsoftening tough hydrogel
相关链接	[Scopus记录]
收录类别	SCI
语种	英语
重要成果	NI期刊 ; NI论文
学校署名	其他
WOS记录号	WOS:000637398300020
ESI学科分类	BIOLOGY & BIOCHEMISTRY ; CLINICAL MEDICINE ; MULTIDISCIPLINARY ; PLANT & ANIMAL SCIENCE ; ENVIRONMENT/ECOLOGY ; SOCIAL SCIENCES, GENERAL ; MICROBIOLOGY ; ECONOMICS BUSINESS ; IMMUNOLOGY ; MATERIALS SCIENCE ; MATHEMATICS ; SPACE SCIENCE ; MOLECULAR BIOLOGY & GENETICS ; PHARMACOLOGY & TOXICOLOGY ; CHEMISTRY ; PSYCHIATRY/PSYCHOLOGY ; NEUROSCIENCE & BEHAVIOR ; PHYSICS ; GEOSCIENCES ; AGRICULTURAL SCIENCES ; ENGINEERING
Scopus记录号	2-s2.0-85103609851
来源库	Scopus
引用统计	被引频次[WOS]：21
成果类型	期刊论文
条目标识符	//www.snoollab.com/handle/2SGJ60CL/222638
专题	工学院_力学与航空航天工程系
作者单位	1.Global Institution for Collaborative Research and Education,Hokkaido University,Sapporo,001-0021,Japan 2.Institute for Chemical Reaction Design and Discovery, Hokkaido University, 001-0021 Sapporo, Japan; gong@sci.hokudai.ac.jp 3.Department of Mechanics and Aerospace Engineering,Southern University of Science and Technology,Shenzhen,518055,China 4.Graduate School of Life Science,Hokkaido University,Sapporo,001-0021,Japan 5.Soft Matter Science and Engineering,City of Paris Industrial Physics and Chemistry Higher Educational Institution (ESPCI Paris),Paris Sciences et Lettres University (PSL),Sorbonne University,CNRS,Paris,75005,France 6.Institute for Chemical Reaction Design and Discovery,Hokkaido University,Sapporo,001-0021,Japan 7.Faculty of Advanced Life Science,Hokkaido University,Sapporo,001-0021,Japan 8.Global Institution for Collaborative Research and Education, Hokkaido University, 001-0021 Sapporo, Japan; kpcui@sci.hokudai.ac.jp gong@sci.hokudai.ac.jp
推荐引用方式 GB/T 7714	Ye，Ya Nan,Cui，Kunpeng,Hong，Wei,et al. Molecular mechanism of abnormally large nonsoftening deformation in a tough hydrogel[J]. Proceedings of the National Academy of Sciences of the United States of America,2021,118(14).
APA	Ye，Ya Nan.,Cui，Kunpeng.,Hong，Wei.,Li，Xueyu.,Yu，Chengtao.,...&Gong，Jian Ping.(2021).Molecular mechanism of abnormally large nonsoftening deformation in a tough hydrogel.Proceedings of the National Academy of Sciences of the United States of America,118(14).
MLA	Ye，Ya Nan,et al."Molecular mechanism of abnormally large nonsoftening deformation in a tough hydrogel".Proceedings of the National Academy of Sciences of the United States of America 118.14(2021).